Browsing by Subject "Detector"
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Item Determination of fission product yields of 235U using gamma ray spectroscopy(2012-12) Lu, Christopher Hing; Biegalski, Steven R.; Landsberger, SheldonIt is important to have a method of experimentally calculating fission product yields. Statistical calculations and simulations produce very large uncertainties. Experimental calculations, depending on the methods used, tend to produce lower uncertainties. This work set up a method to calculate fission product yields using gamma ray spectroscopy. In order to produce a method that was theoretically sound, a simulation was set up using OrigenArp to calculate theoretical concentrations of fission products from the irradiation of natural uranium. From these concentrations, the fission product yields were calculated to verify that they would agree with expected values. Moving forward in the work, the total flux at the point of irradiation, in the pneumatic transfer system, was calculated and determined to be 3.9070E+11 ± 6.9570E+10 n/cm^2/s at 100 kW. Once the flux was calculated, the method for calculating fission product yields was implemented and yields were calculated for 10 fission products. The yields calculated were in very good agreement (within 10.04%) with expected values taken from the ENDF-349 library. This method has strong potential in nuclear forensics as it can provide a means for developing a library of experimentally-determined fission product yields, as well as rapid post-nuclear detonation analysis.Item Multispectral gamma-ray analysis using clover detectors with application to uranium fission product analysis(2013-05) Horne, Steven Michael; Landsberger, Sheldon; Jackman, Kevin RichardA high-efficiency gamma-ray counting system has been built at Los Alamos National Laboratory for use in analyzing nuclear forensics samples. This system consists of two clover high-purity germanium detectors and is surrounded by a thallium-doped sodium iodide annulus. Special precautions have been taken to ensure the system has a low background. The system is connected to XIA Pixie-4 fast digitizers and collects data in list-mode. This work is split into two main parts. The first part describes the proper steps and techniques to initialize the settings of a detector system connected to fast digitizers in order to optimize the system for resolution and throughput. The various counting modes for this particular system are described in detail, including the benefits and drawbacks of each mode. Steps are then shown to characterize the system by obtaining efficiency curves for various counting modes and sample geometries. Because of the close counting geometry involved with this system, true-coincidence summing factors must be calculated, and are done so in part by measuring the peak-to-total ratios of the system in its various counting modes across a wide energy range. The dead-time for the system can be complicated due to the multiple inputs of the system. Techniques for calculating the dead-time of multiple-detector systems are discussed. The second part of this work shows the system's usefulness in analyzing nuclear forensics samples, specifically irradiated enriched uranium. Three fission product parent-daughter pairs of different lifetimes are analyzed over a course of six months. The activities of each nuclide are calculated at each time step. Age dating techniques using the parent-daughter pairs are discussed, as well as the detection limits of each nuclide for a range of sample ages. Finally, avenues for further research are presented, as well as potential sources of error or uncertainty for this work.Item Wavelength selective and 3D stacked microbolometers for multispectral infrared detection(2012-05) Park, Jong Yeon; Neikirk, Dean P., 1957-; Bank, Seth; Dodabalapur, Ananth; Hall, Neal; Shi, LiDevelopment of wavelength selective detection, tunable multi-spectral capability with functionality in the infrared spectral region is highly desirable for a variety of applications such as thermography, chemical processing and environmental monitoring, spectroradiometry, medical diagnosis, Fourier transform infrared spectroscopy, night vision, mine detection, military defense and astronomy. Infrared detector with wavelength selective functionality have emerged as next generation infrared detectors. This study presents fabrication and characterization of wavelength selective Germanium dielectric coated Salisbury screen and novel 3D stacked microbolometer for multispectral infrared detection. This novel fabrication process helps produce much flatter, more robust device structure by using an un-patterned sacrificial layer to produce device legs that hold the central structural layer above the reflective mirror supported by a completely flat sacrificial layer with sufficient thermal isolation to allow microbolometer operation. For the fabricated wavelength selective Germanium dielectric coated Salisbury screen microbolometer using self aligned process, the FTIR measured spectral responses and numerical simulation results show excellent agreement with wavelength selectivity (9[mu]m, 10[mu]m, 11[mu]m) in long wave infrared (LWIR) region. To achieve multicolor infrared detection, recently a few device concepts using uncooled detectors have been reported. However, none of the proposed device designs have demonstrated fabrication. Moreover, Commercial Fabry-perot resonant cavity based uncooled microbolometers (Air gap: 2 to 2.5μm) have limited design parameters due to multicolor narrow band spectral response. In this study, a feasible device fabrication method for novel 3D stacked microbolometer is demonstrated for multispectral uncooled infrared detector that can achieve tunable narrowband absorption in mid-wave infrared (MWIR) and long-wave infrared (LWIR) spectral regions.